Article
Conformational Dynamics of Bacteriochlorophyll c in Chlorosomes from the bchQ Mutant of Chlorobaculum tepidum.
The journal of physical chemistry. B - 27 Feb 2025
Dsouza Lolita, Gupta Karthick Babu Sai Sankar, Li Xinmeng, Erić Vesna, Luo Yusen, Huijser Annemarie, Jansen Thomas L C, Buda Francesco, Holzwarth Alfred R, Bryant Donald A, Gurinov Andrei, Sevink G J Agur, de Groot Huub J M
Abstract excerpt
In contrast to the common viewpoint that bacteriochlorophyll (BChl) motion is largely absent within the chlorosome assembly, physics-based modeling points to a crucial role of the nanoscale librational motion of the macrocycle for the transfer of excitons. To elucidate this motion experimentally, compositional uniformity and high sensitivity are required. We focused on uniformly 13C labeled chlorosome...
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