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Article

Probing the Effect of Mutations on Light Harvesting in CP29 by Transient Absorption and First-Principles Simulations.

The journal of physical chemistry letters - 20 Jun 2024

Saraceno Piermarco, Sardar Samim, Caferri Roberto, Camargo Franco V A, Dall'Osto Luca, D'Andrea Cosimo, Bassi Roberto, Cupellini Lorenzo, Cerullo Giulio, Mennucci Benedetta

Abstract excerpt

Natural light harvesting is exceptionally efficient thanks to the local energy funnel created within light-harvesting complexes (LHCs). To understand the design principles underlying energy transport in LHCs, ultrafast spectroscopy is often complemented by mutational studies that introduce perturbations into the excitonic structure of the natural complexes. However, such studies may fall short of identifying all...

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PMID: 38861672
DOI: 10.1021/acs.jpclett.4c01040

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